Quantum-Enhanced Nonlinear Spectroscopy

Nonfiction, Science & Nature, Science, Physics, Spectrum Analysis, Optics
Cover of the book Quantum-Enhanced Nonlinear Spectroscopy by Frank Schlawin, Springer International Publishing
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Author: Frank Schlawin ISBN: 9783319443973
Publisher: Springer International Publishing Publication: September 10, 2016
Imprint: Springer Language: English
Author: Frank Schlawin
ISBN: 9783319443973
Publisher: Springer International Publishing
Publication: September 10, 2016
Imprint: Springer
Language: English

This thesis focuses on nonlinear spectroscopy from a quantum optics perspective. First, it provides a detailed introduction to nonlinear optical signals; starting from Glauber’s photon counting formalism, it establishes the diagrammatic formulation, which forms the backbone of nonlinear molecular spectroscopy.

 

The main body of the thesis investigates the impact of quantum correlations in entangled photon states on two-photon transitions, with a particular focus on the time-energy uncertainty, which restricts the possible simultaneous time and frequency resolution in measurements. It found that this can be violated with entangled light for individual transitions. The thesis then presents simulations of possible experimental setups that could exploit this quantum advantage.

 

The final chapter is devoted to an application of the rapidly growing field of multidimensional spectroscopy to trapped ion chains, where it is employed to investigate nonequilibrium properties in quantum simulations.

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This thesis focuses on nonlinear spectroscopy from a quantum optics perspective. First, it provides a detailed introduction to nonlinear optical signals; starting from Glauber’s photon counting formalism, it establishes the diagrammatic formulation, which forms the backbone of nonlinear molecular spectroscopy.

 

The main body of the thesis investigates the impact of quantum correlations in entangled photon states on two-photon transitions, with a particular focus on the time-energy uncertainty, which restricts the possible simultaneous time and frequency resolution in measurements. It found that this can be violated with entangled light for individual transitions. The thesis then presents simulations of possible experimental setups that could exploit this quantum advantage.

 

The final chapter is devoted to an application of the rapidly growing field of multidimensional spectroscopy to trapped ion chains, where it is employed to investigate nonequilibrium properties in quantum simulations.

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